Enaminone-Directed Rh(III)-Catalyzed Hydroarylation Reaction of Oxa/azabenzonorbornadienes through C-H Bond Functionalization

Jitendra D. Belani; Milind M Ahire

doi:10.1055/a-2685-9449

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Synlett
DOI: 10.1055/a-2685-9449

Letter

Enaminone-Directed Rh(III)-Catalyzed Hydroarylation Reaction of Oxa/azabenzonorbornadienes through C-H Bond Functionalization

Jitendra D. Belani

¹Pharmaceutical Sciences, College of Pharmacy, Thomas Jefferson University, Philadelphia, United States (Ringgold ID: RIN6559)

,

Milind M Ahire

¹Pharmaceutical Sciences, College of Pharmacy, Thomas Jefferson University, Philadelphia, United States (Ringgold ID: RIN6559)

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We report a Rh(III)-catalyzed hydroarylation of oxa-and azabenzonorbornadienes directed by enaminones through C-H activation. The reaction proceeds under mild conditions with broad substrate scope and excellent regioselectivity. Diverse polycyclic products are obtained in high yields. A representative structure was confirmed by X-ray analysis.

Publikationsverlauf

Eingereicht: 25. Juli 2025

Angenommen nach Revision: 18. August 2025

Accepted Manuscript online:
19. August 2025

Georg Thieme Verlag KG
Oswald-Hesse-Straße 50, 70469 Stuttgart, Germany